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The Do&Co Albertina has everything you are looking for if you want to go somewhere where the food is great, the atmposphere is special and cozy, the decor is modern and upscale and, last but not least, the service is excellent. You will find it here.
If the weather allows it - try and find a place in on the terrace overlooking the Palmenhaus and the Burggarten - it is very peaceful and you have beautiful views.
The menu hold something for everybody - international, Italian, but also typical Viennese dishes (they are really deliciously prepared here) - and if you really cannot find anything - go for the Spanish tapas to nibble on - they are not like the ones you will get in Spain, but close enough....
But the one thing you should not miss here: the Mohr im Hemd (Viennese desert - warm chocolate/nut soufflee surrounded with whipped cream) - you will rarely be able to taste a better version than here.
Do&Co Albertina is also great place to just have coffee on the terrace, or a drink at their trendy bar. Customers tend to be more on the 'middleaged and settled' side, but the atmosphere is still classy and modern at the same time!